Tag Archives: Leonid Levitov

A new wave of physics: electrons flow like liquid in graphene

Unfortunately I couldn’t find a credit for the artist for the graphic (I really like it) which accompanies the news about a new physics and graphene,

Courtesy: University of Manchester

From an Aug. 22, 2017 news item on phys.org (Note: A link has been removed),

A new understanding of the physics of conductive materials has been uncovered by scientists observing the unusual movement of electrons in graphene.

Graphene is many times more conductive than copper thanks, in part, to its two-dimensional structure. In most metals, conductivity is limited by crystal imperfections which cause electrons to frequently scatter like billiard balls when they move through the material.

Now, observations in experiments at the National Graphene Institute have provided essential understanding as to the peculiar behaviour of electron flows in graphene, which need to be considered in the design of future Nano-electronic circuits.

An Aug. 22, 2017 University of Manchester press release, which originated the news item, delves further into the research (Note: Links have been removed),

Appearing today in Nature Physics, researchers at The University of Manchester, in collaboration with theoretical physicists led by Professor Marco Polini and Professor Leonid Levitov, show that Landauer’s fundamental limit can be breached in graphene. Even more fascinating is the mechanism responsible for this.

Last year, a new field in solid-state physics termed ‘electron hydrodynamics’ generated huge scientific interest. Three different experiments, including one performed by The University of Manchester, demonstrated that at certain temperatures, electrons collide with each other so frequently they start to flow collectively like a viscous fluid.

The new research demonstrates that this viscous fluid is even more conductive than ballistic electrons. The result is rather counter-intuitive, since typically scattering events act to lower the conductivity of a material, because they inhibit movement within the crystal. However, when electrons collide with each other, they start working together and ease current flow.

This happens because some electrons remain near the crystal edges, where momentum dissipation is highest, and move rather slowly. At the same time, they protect neighbouring electrons from colliding with those regions. Consequently, some electrons become super-ballistic as they are guided through the channel by their friends.

Sir Andre Geim said: “We know from school that additional disorder always creates extra electrical resistance. In our case, disorder induced by electron scattering actually reduces rather than increase resistance. This is unique and quite counterintuitive: Electrons when make up a liquid start propagating faster than if they were free, like in vacuum”.

The researchers measured the resistance of graphene constrictions, and found it decreases upon increasing temperature, in contrast to the usual metallic behaviour expected for doped graphene.

By studying how the resistance across the constrictions changes with temperature, the scientists revealed a new physical quantity which they called the viscous conductance. The measurements allowed them to determine electron viscosity to such a high precision that the extracted values showed remarkable quantitative agreement with theory.

Here’s a link to and a citation for the paper,

Superballistic flow of viscous electron fluid through graphene constrictions by R. Krishna Kumar, D. A. Bandurin, F. M. D. Pellegrino, Y. Cao, A. Principi, H. Guo, G. H. Auton, M. Ben Shalom, L. A. Ponomarenko, G. Falkovich, K. Watanabe, T. Taniguchi, I. V. Grigorieva, L. S. Levitov, M. Polini, & A. K. Geim. Nature Physics (2017) doi:10.1038/nphys4240 Published online 21 August 2017

This paper is behind a paywall.

Graphene like water

This is graphene research from Harvard University and Raytheon according to a Feb. 11, 2016 news item on phys.org (Note: Links have been removed),

It’s one atom thick [i.e., two-dimensional], stronger than steel, harder than diamond and one of the most conductive materials on earth.

But, several challenges must be overcome before graphene products are brought to market. Scientists are still trying to understand the basic physics of this unique material. Also, it’s very challenging to make and even harder to make without impurities.

In a new paper published in Science, researchers at the [sic] Harvard and Raytheon BBN Technology have advanced our understanding of graphene’s basic properties, observing for the first time electrons in a metal behaving like a fluid.

A Feb. 11, 2016 Harvard University press release by Leah Burrows (also on EurekAlert), which originated the news item, provides more detail,

In order to make this observation, the team improved methods to create ultra-clean graphene and developed a new way measure its thermal conductivity. This research could lead to novel thermoelectric devices as well as provide a model system to explore exotic phenomena like black holes and high-energy plasmas.

An electron super highway

In ordinary, three-dimensional metals, electrons hardly interact with each other. But graphene’s two-dimensional, honeycomb structure acts like an electron superhighway in which all the particles have to travel in the same lane. The electrons in graphene act like massless relativistic objects, some with positive charge and some with negative charge. They move at incredible speed — 1/300 of the speed of light — and have been predicted to collide with each other ten trillion times a second at room temperature.  These intense interactions between charge particles have never been observed in an ordinary metal before.

The team created an ultra-clean sample by sandwiching the one-atom thick graphene sheet between tens of layers of an electrically insulating perfect transparent crystal with a similar atomic structure of graphene.

“If you have a material that’s one atom thick, it’s going to be really affected by its environment,” said Jesse Crossno, a graduate student in the Kim Lab [Philip Kim, professor of physics and applied physics] and first author of the paper.  “If the graphene is on top of something that’s rough and disordered, it’s going to interfere with how the electrons move. It’s really important to create graphene with no interference from its environment.”

The technique was developed by Kim and his collaborators at Columbia University before he moved to Harvard in 2014 and now have been perfected in his lab at SEAS [Harvard School of Engineering and Applied Sciences].

Next, the team set up a kind of thermal soup of positively charged and negatively charged particles on the surface of the graphene, and observed how those particles flowed as thermal and electric currents.

What they observed flew in the face of everything they knew about metals.

A black hole on a chip

Most of our world — how water flows or how a curve ball curves —  is described by classical physics. Very small things, like electrons, are described by quantum mechanics while very large and very fast things, like galaxies, are described by relativistic physics, pioneered by Albert Einstein.

Combining these laws of physics is notoriously difficult but there are extreme examples where they overlap. High-energy systems like supernovas and black holes can be described by linking classical theories of hydrodynamics with Einstein’s theories of relativity.

But it’s difficult to run an experiment on a black hole. Enter graphene.

When the strongly interacting particles in graphene were driven by an electric field, they behaved not like individual particles but like a fluid that could be described by hydrodynamics.

“Instead of watching how a single particle was affected by an electric or thermal force, we could see the conserved energy as it flowed across many particles, like a wave through water,” said Crossno.

“Physics we discovered by studying black holes and string theory, we’re seeing in graphene,” said Andrew Lucas, co-author and graduate student with Subir Sachdev, the Herchel Smith Professor of Physics at Harvard. “This is the first model system of relativistic hydrodynamics in a metal.”

Moving forward, a small chip of graphene could be used to model the fluid-like behavior of other high-energy systems.

Industrial implications

So we now know that strongly interacting electrons in graphene behave like a liquid — how does that advance the industrial applications of graphene?

First, in order to observe the hydrodynamic system, the team needed to develop a precise way to measure how well electrons in the system carry heat.  It’s very difficult to do, said co-PI Kin Chung Fong, scientist with Raytheon BBN Technology.

Materials conduct heat in two ways: through vibrations in the atomic structure or lattice; and carried by the electrons themselves.

“We needed to find a clever way to ignore the heat transfer from the lattice and focus only on how much heat is carried by the electrons,” Fong said.

To do so, the team turned to noise. At finite temperature, the electrons move about randomly:  the higher the temperature, the noisier the electrons. By measuring the temperature of the electrons to three decimal points, the team was able to precisely measure the thermal conductivity of the electrons.

“This work provides a new way to control the rate of heat transduction in graphene’s electron system, and as such will be key for energy and sensing-related applications,” said Leonid Levitov, professor of physics at MIT [Massachusetts Institute of Technology].

“Converting thermal energy into electric currents and vice versa is notoriously hard with ordinary materials,” said Lucas. “But in principle, with a clean sample of graphene there may be no limit to how good a device you could make.”

Here’s a link to and a citation for the paper,

Observation of the Dirac fluid and the breakdown of the Wiedemann-Franz law in graphene by Jesse Crossno, Jing K. Shi, Ke Wang, Xiaomeng Liu, Achim Harzheim, Andrew Lucas, Subir Sachdev, Philip Kim, Takashi Taniguchi, Kenji Watanabe, Thomas A. Ohki, Kin Chung Fong.Science  11 Feb 2016: pp. DOI: 10.1126/science.aad0343

This paper is behind a paywall.

Here’s an image illustrating the research,

Caption: In a new paper published in Science, researchers at the Harvard and Raytheon BBN Technology have advanced our understanding of graphene's basic properties, observing for the first time electrons in a metal behaving like a fluid. Credit: Peter Allen/Harvard SEAS

Caption: In a new paper published in Science, researchers at the Harvard and Raytheon BBN Technology have advanced our understanding of graphene’s basic properties, observing for the first time electrons in a metal behaving like a fluid. Credit: Peter Allen/Harvard SEAS